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Abstract: The effect of state-selective reactive decay on the relaxation kinetics ofquantum multistate systems is studied in detail in the Bloch-Redfield approachBRA. The results are applied to the analysis of this effect in radical pairrecombination kinetics. The BRA is shown to be able to describe quantitativelymost important specific features of the recombination kinetics including thosepredicted by phenomenological treatment and by recently proposed approachesbased on quantum measurement theories.



Autor: A. I. Shushin

Fuente: https://arxiv.org/







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