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 High-order harmonic generation from field-distorted orbitals


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We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results allow us to suggest that field-distortion is the reason why the two-center interference minimum has never been observed experimentally in N2. We propose experimental parameters which should allow an observation of the two-center interference minimum.



Author: Maciej Dominik Śpiewanowski; Adam Etches; Lars Bojer Madsen

Source: https://archive.org/







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