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Abstract : A theory of vibrational energy transfer using long-range multipolar interaction has been extended to the case of a transfer between a diatomic and a symmetric top molecule. Energy transfer probabilities versus temperature were calculated for five energy-exchange reactions between D2V = 1 and CH3Cl, CH3CCH or NH3. Due to the great number of rotational levels in symmetric top molecules, the values obtained are rather low.

Keywords : ammonia deuterium molecular inelastic collisions molecular rotational vibrational energy transfer organic compounds near resonant molecular collisions symmetric top molecules vibrational energy transfer long range multipolar interaction probabilities energy exchange reactions D sub 2 NH sub 3 rotational levels diatomic molecules allylene chloromethane





Autor: L. Torchin

Fuente: https://hal.archives-ouvertes.fr/



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